A note: I vastly prefer subtitled anime, as the voice acting is far more emptional and poingant in Japanese. However, there have been some excellent American dubs (the new Akira, for example).
All-time favs:
Akira (all versions)
FLCL (Fooley Cooley) - freakin' awesome spasticity!
Ghost in the Shell (1st movie)
Giant Robo (if you haven't seen this series, do so!)
Irresponsible Captain Tylor
Princess Mononoke (beautiful)
Trigun
Other Anime:
Bastard!
Battle Angel Alita
Big O
Blue Submarine #6
Cowboy Bebop
Dominion Tank Police
Dragon Ball Z (some episodes)
Fist of the North Star (ultracheese, and the worst ending ever!)
Galaxy Express 999, Queen Emeraldas, and two of Captain Harlock's movies
Golgo13: The Professional
Gundam Wing (some episodes)
Pokemon 
Ranma 1/2 (some of the first episodes)
Record of Lodoss War
Robot Carnival
Robotech (American bastardized version - saw it as a kid, 3 times)
Rurouni Kenshin
Sailor Moon (some episodes)
Slayers (some of the first episodes)
Tenchi Muyo (original series)
Urotsokedoje - Legend of the Overfiend
Vampire Hunter D - original
Vampire Hunter D: Bloodlust
Non-Japanese animation:
Animatrix
Aqua Teen Hunger Force
Brak Presents the Brak Show Starring Brak
Disney - All main movies (not sequels)
G.I. Joe (original series and movie)
Happy Tree Friends
Heavy Metal (awesome!)
Heavy Metal FAKK 2000 (crap!)
Ren & Stimpy (the originals by John Krikfalusi)
Road to El Dorado
Sealab 2021
South Park
Space Ghost Coast to Coast (and other related weirdness)
Transformers (original series & the terribly cheesy movie)
Um.... that's all I can think of off the top of my head... 
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